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The logistics associated with the coffee wastes supply chain need to be carefully evaluated to provide economic and environmental sustainability along the entire life cycle of coffee wastes used as raw materials.
Another interesting conceptualization of spent coffee ground biorefinery was based on different approaches to make products, separating primary products which are obtained by the already discussed fractionation, and secondary products obtained by their transformation through biotechnological, chemical, and thermochemical routes. These secondary products include bioprocessing products (lactic acid, PHAs, biogas, triglycerides from yeast, bioethanol), biodiesel, fertilizers, animal feeds, formulations of polysaccharides and antioxidants (mainly for cosmetics), biosorbents, and biodegradable films for food packaging and construction materials.15 A critical point for the economic viability of a spent coffee biorefinery is definitely the logistics for the supply and recovery of SCGs. Moreover, many of the processes must take into account the presence of contaminants and the overall lifecycle of the processing to ensure a low impact of the biorefinery product. Coupling high added value chemical isolations with thermochemical valorization for energy and materials recovery seems to emerge as a reasonable approach to be further explored and investigated.10,11,12,13,14,15,16 Thermochemical valorization leads to mainly bio-oils and bio-chars, and minor quantities of biogas through hydrothermal or pyrolytic processes. Clearly the process conditions are varied to maximize the desired output of oil, char, and gas for the intended circular economy approach.15,16 As better detailed in the next section, the solid carbon fraction (char) obtained by thermal treatment of spent coffee grounds can be further chemically or physically activated at high temperatures to produce carbon materials with high surface area and controlled porosity (activated carbon) with key properties as active materials for electrochemical energy storage and conversion devices. This is one of the most intriguing emerging applications to re-use coffee waste and specifically spent coffee grounds by valorizing their intrinsic chemical and physical properties.
One of the main aspects to be carefully evaluated, which is common to any circular economy model, is the logistics of the coffee waste supply, to actually provide an economic and environmental sustainability along the entire life cycle.
A comparison with technological, economic, and environmental benefits of alternatives in the strategies required for using recycled energy storage device materials is strongly needed. Nonetheless, despite the open challenges, the feasibility of using coffee waste for electrochemical energy storage represents an opportunity to create a second energizing life for coffee used in our daily life, by building new circular value chains and ecosystems.
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